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• W2090962338 abstract "We study macroion correlation effects on the thermodynamics of highly charged colloidal suspensions using a mean-field theory and primitive model computer simulations. We suggest a simple way to include the macroion correlations into the mean-field theory as an extension of the renormalized jellium model of Trizac and Levin [Phys. Rev. E {bf 69}, 031403 (2004)]. The effective screening parameters extracted from our mean-field approach are then used in a one-component model with macroions interacting via Yukawa-like potential to predict macroion distributions. We find that inclusion of macroion correlations leads to a weaker screening and hence smaller effective macroion charge and lower osmotic pressure of the colloidal dispersion as compared to other mean-field models. This result is supported by a comparison to primitive model simulations and experiments for charged macroions in the low-salt regime, where the macroion correlations are expected to be significant." @default.
• W2090962338 created "2016-06-24" @default.
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• W2090962338 date "2006-11-28" @default.
• W2090962338 modified "2023-10-07" @default.
• W2090962338 title "Macroion correlation effects in electrostatic screening and thermodynamics of highly charged colloids" @default.
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• W2090962338 doi "https://doi.org/10.1103/physreve.74.051408" @default.
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