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• W2091240742 abstract "Scanning tunneling spectroscopy (STS) allows to image single molecules decoupled from the supporting substrate. The obtained images are routinely interpreted as the square moduli of molecular orbitals, dressed by the mean-field electron-electron interaction. Here we demonstrate that the effect of electron correlation beyond mean field qualitatively alters the uncorrelated STS images. Our evidence is based on the ab-initio many-body calculation of STS images of planar molecules with metal centers. We find that many-body correlations alter significantly the image spectral weight close to the metal center of the molecules. This change is large enough to be accessed experimentally, surviving to molecule-substrate interactions." @default.
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• W2091240742 date "2013-01-03" @default.
• W2091240742 modified "2023-10-16" @default.
• W2091240742 title "Proposed Alteration of Images of Molecular Orbitals Obtained Using a Scanning Tunneling Microscope as a Probe of Electron Correlation" @default.
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• W2091240742 doi "https://doi.org/10.1103/physrevlett.110.018305" @default.
• W2091240742 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/23383849" @default.
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