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- W2091255981 abstract "We have investigated the electron phase-memory relaxation time of the nitroxyl radical 2,2,6,6-tetramethylpiperidine-1-oxyl at temperatures between 5 and 80 K in crystalline and glassy states of ethanol using pulsed X-band electron paramagnetic resonance spectroscopy. The results indicate that the transition from the slow to fast motion regimes of the paramagnetic center occurs upon further cooling of the sample below ∼20 K. We provide experimental evidence that this phenomenon cannot be ascribed to the impact of hyperfine interactions with methyl protons in the system, but it can be instead a signature of the coupling of the electron spin with the boson peak excitations of the lattice." @default.
- W2091255981 created "2016-06-24" @default.
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- W2091255981 date "2011-01-28" @default.
- W2091255981 modified "2023-09-27" @default.
- W2091255981 title "Fast motion in molecular solids at low temperatures: Evidence from a pulsed electron paramagnetic resonance study of nitroxyl radical relaxation" @default.
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- W2091255981 doi "https://doi.org/10.1063/1.3533798" @default.
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