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- W2091275120 abstract "The glass transition in dipolar glass formers with long-range indirect dipole-dipole interactions has been studied by Monte Carlo simulation. Our simulation shows that the non-Arrhenien behavior of the relaxation time with temperature is induced by a progressive crossover from a regime of fast dynamics at high temperature in the polar liquid to one of slow dynamics controlled by the presence of polar clusters. The interaction between the clusters results in a spectrum of relaxation time and transition to the glass state. The glass transition starts at a temperature ${T}_{0}>{T}_{mathrm{c}}$, below which spatial heterogeneities appear. These spatial heterogeneities start to influence the dynamical behavior and the spectrum of relaxation time becomes asymmetric. Below ${T}_{mathrm{c}}$, when the polar clusters reach a nanometric size ergodicity breaking occurs." @default.
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- W2091275120 date "2007-02-01" @default.
- W2091275120 modified "2023-10-16" @default.
- W2091275120 title "Monte Carlo simulation of cooperative orientation relaxation of dipoles in glass formers" @default.
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- W2091275120 doi "https://doi.org/10.1103/physrevb.75.054102" @default.
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