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• W2091465610 abstract "The adsorption of acetic acid is studied as a function of gold content by temperature-programmed desorption and reflection–absorption infrared spectroscopy on Au/Pd(1 1 1) alloys formed by depositing 5 ML of gold onto a Pd(1 1 1) surface and heating to various temperatures. For mole fractions of gold greater than ∼0.5, acetic acid adsorbs molecularly and desorbs intact with an activation energy of ∼52 kJ/mol. This acetic acid is present as catemers, where the nature of the catemer is found to depend on gold concentration. When the relative gold concentration is less than ∼0.33, adsorption of acetic acid at 80 K and heating to ∼207 K forms η1-acetate species on the surface. On further heating, these can either thermally decompose to eventually evolve hydrogen, water and oxides of carbon, or form η2-acetate species, where the coverage of reactively formed η2-acetate species increases with decreasing gold concentration in the near surface region." @default.
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• W2091465610 date "2007-03-01" @default.
• W2091465610 modified "2023-10-17" @default.
• W2091465610 title "The adsorption of acetic acid on Au/Pd(1 1 1) alloy surfaces" @default.
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• W2091465610 doi "https://doi.org/10.1016/j.susc.2006.12.079" @default.
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