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- W2091567328 abstract "Abstract In order to avoid a rather laborious extension of the treatment of Wang Chang, Uhlenbeck and De Boer to mixtures where the rate of exchange between translational and internal energy is slow, we developed a phenomenological treatment based on thermodynamics of irreversible processes. We introduced new expressions for the diffusion and thermal diffusion coefficients, which account for this exchange in the case of a local equilibrium between the rotational states of diatomic component in a mixture with an inert gas. We made use of the concept in which the internal degrees of freedom are considered as chemically reacting components. The multicomponent diffusion coefficients occuring in the new expressions were related to the newly calculated collision integrals based on the transport cross sections obtained in the preceding paper∗) for the system HT-He. The agreement between the theoretical diffusion and thermal diffusion coefficients for this mixture is much improved as compared to earlier attempts." @default.
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- W2091567328 date "1967-01-01" @default.
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- W2091567328 title "Diffusion and thermal diffusion in gaseous mixtures with internal degrees of freedom" @default.
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- W2091567328 doi "https://doi.org/10.1016/0031-8914(67)90094-8" @default.
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