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- W2091962034 abstract "Abstract The quasi-thermodynamic description of the adsorption from binary mixtures described in Part I for the liquid—vapour interface has been applied in this paper to the boundary between mercury electrode and dilute electrolyte solution in binary solvent. Theoretical surface tension—composition curves for uncharged Hg were calculated and compared with the experimental data for H2O + methanol, acetone, sulpholane and dimethylsulphoxide mixtures. For this the two adjustable parameters of the isotherm were needed: τ, the thickness of the surface phase and K, the degree of non-ideality of mixing in the phase as compared with that in the bulk liquid. The parameters found for all systems as well for the free surface as for Hg—solution interface were as follows: τ was almost always somewhat larger than the thickness of the monomolecular layer of organic component and K was somewhat less than unity. This indicates that the non-ideality in the surface phase is always smaller than in the bulk. The agreement between the calculated and experimental values was reasonably good. It has been found that the isotherm can be described with the same parameters also for other charges or potentials in a given range of q or E depending on the organic component. The method of the calculation of electrocapillary curves has been also described." @default.
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- W2091962034 date "1975-10-10" @default.
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- W2091962034 title "Adsorption at fluid interfaces II. Surface tension at the interface between a binary liquid mixture and an ideal polarized mercury electrode," @default.
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- W2091962034 doi "https://doi.org/10.1016/0368-1874(75)85158-6" @default.
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