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- W2092124372 abstract "Photoexcited states in transpolyacetylene [t-(CH${)}_{mathit{x}}$], and in alkoxy derivatives of poly(paraphenylenevinylene) (PPV) nondegenerate ground-state polymers, have been studied by the technique of absorption detected magnetic resonance. In addition to the stable charged photoexcitations, which are charged solitons in t-(CH${)}_{mathit{x}}$ and bipolarons in PPV, we clearly identify neutral photoexcitations with nonzero spins. In t-(CH${)}_{mathit{x}}$ these are spin-1/2 neutral solitons ${mathit{S}}^{0}$(Sifmmodebarelsetextasciimacronfi{} $^{0}$) with an optical transition at 1.35 eV. The neutral photoexcitations in PPV form triplet excitons which cannot dissociate into ${mathit{S}}^{0}$Sifmmodebarelsetextasciimacronfi{} $^{0}$ pairs due to the confinement caused by the nondegenerate backbone structure." @default.
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- W2092124372 date "1992-02-03" @default.
- W2092124372 modified "2023-09-26" @default.
- W2092124372 title "Studies of photoexcited states in polyacetylene and poly(paraphenylenevinylene) by absorption detected magnetic resonance: The case of neutral photoexcitations" @default.
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- W2092124372 doi "https://doi.org/10.1103/physrevlett.68.666" @default.
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