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• W2092257023 abstract "A metal-semiconductor transition at ${mathit{T}}_{mathit{c}}$=170.4 K in a two-dimensional organic metal, (BEDT-TTF${)}_{3}$(${mathrm{ClO}}_{4}$${)}_{2}$, was investigated by means of ESR, resistivities, specific heats, and x-ray diffractions. The specific heats show a ensuremath{lambda}-type anomaly at ${mathit{T}}_{mathit{c}}$ with a second-order nature and a large entropy change range of 3 J/K mol. In addition to the H/D isotope effects on ${mathit{T}}_{mathit{c}}$, x-ray diffraction suggests the development of an intermolecular interaction network between the ethylene groups of BEDT-TTF molecules and ${mathrm{ClO}}_{4}^{mathrm{ensuremath{-}}}$ anions below ${mathit{T}}_{mathit{c}}$. These experimental findings demonstrate that the three-dimensional structural rearrangement, which is closely correlated to the development of the intermolecular interaction network, plays an important role in the metal-semiconductor transition." @default.
• W2092257023 created "2016-06-24" @default.
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• W2092257023 date "1994-12-01" @default.
• W2092257023 modified "2023-10-17" @default.
• W2092257023 title "Metal-semiconductor transition and structural change in (BEDT-TTF<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:mrow><mml:msub><mml:mrow><mml:mo>)</mml:mo></mml:mrow><mml:mrow><mml:mn>3</mml:mn></mml:mrow></mml:msub></mml:mrow></mml:math>(<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:mrow><mml:msub><mml:mrow><mml:mi mathvariant=normal>ClO</mml:mi></mml:mrow><mml:mrow><mml:mn>4</mml:mn></mml:mrow></mml:msub></mml:mrow></mml:math…" @default.
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• W2092257023 doi "https://doi.org/10.1103/physrevb.50.16287" @default.
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