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- W2092357601 abstract "Three-pulse photon-echo peak-shift (3PEPS) experiments were performed to explore structural relaxations relevant to solvation of a cyanine dye non-covalently anchored to aqueous interfaces of unilamellar phospholipid vesicles. The influence of the lipid polymorphism is studied through the temperature-dependence of the 3PEPS decay. As opposed to the main order/disorder phase transition connected with packing phenomena in the hydrophobic membrane core, the rippled-to-gel pre-transition strongly affects the solvation response on time scales below 2 ps. This finding indicates that the pre-transition is connected with structural modifications of the hydration shell surrounding the polar head groups and is consistent with a dehydration of the interface." @default.
- W2092357601 created "2016-06-24" @default.
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- W2092357601 date "2002-01-01" @default.
- W2092357601 modified "2023-09-27" @default.
- W2092357601 title "Probing solvation dynamics at aqueous lipid-membrane interfaces with 3-pulse photon-echo peak-shifts" @default.
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- W2092357601 doi "https://doi.org/10.1364/up.2002.wd32" @default.
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