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- W2092416218 abstract "Summary Coprecipitation may be a significant process in controlling radionuclide (RN) release during spent fuel dissolution/reprecipitation in a breached geological disposal site by water. The objective of this work was to study the coprecipitation of thorium with UO 2 as host phase under reducing conditions (pure N 2 and E h <-100 mV/SHE) as a function of pH and [Th]/[U] initial concentration ratio. For pH < 4, the final concentration of Th was found to be considerably lower than expected if pure phase, Th(OH) 4 (s) was formed. Coprecipitation phenomena and formation of solid solutions (U,Th)O 2+x (s) are suggested to be responsible for the lower solubility concentrations. For pH > 4, the final concentrations seems to be similar to pure phase solubility." @default.
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- W2092416218 date "2002-09-01" @default.
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- W2092416218 title "Coprecipitation of thorium with UO<sub>2</sub>" @default.
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- W2092416218 doi "https://doi.org/10.1524/ract.2002.90.9-11_2002.523" @default.
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