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• W2092458046 abstract "The 193 nm photodissociation of the isotopomers SO2, SO*2 and SOO* (with O*=18O) was studied by high-resolution photo-fragment translational spectroscopy. The translational energy distributions P(ET) of the fragment pairs SO+O, SO*+O*, SO+O* and SO*+O were determined from systematic analysis of the time-of-flight distributions obtained with various degrees of O* substitution and were found to be significantly different due to a different ro-vibrational distribution of the diatomic fragments. In the case of the symmetric isotopomers SO2 and SO*2 the difference of the P(ET) distributions is attributed to a slightly different state excitation in the C̃ electronic band of the parent molecule. The SO and SO* bond fission of the asymmetric SO0* have equal probabilities but lead to different energy distributions in the SO and SO* fragments which reflect subtle differences in the dissociation dynamics of the two reaction modes." @default.
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• W2092458046 date "1993-03-01" @default.
• W2092458046 modified "2023-10-17" @default.
• W2092458046 title "Isotope specific photodissociation of SO2 at 193.3 nm" @default.
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• W2092458046 doi "https://doi.org/10.1016/0009-2614(93)90004-k" @default.
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