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- W2092560165 abstract "In pyrite-structure antiferromagnetic ${mathrm{NiS}}_{2}$, the magnetic susceptibility ensuremath{chi}(T) shows downward curvature above the N'eel transition (${mathit{T}}_{mathit{N}1}$=39.2 K), suggesting that magnetic correlations persist to T=400 K. However, neutron-scattering measurements indicate that the bulk magnetic behavior above ${mathit{T}}_{mathit{N}1}$ is conventional. We present evidence that the unusual temperature dependence of ensuremath{chi}(T) arises from a surface contribution. At ${mathit{T}}_{mathit{N}2}$=29.75 K a transition occurs to a weakly ferromagnetic state, accompanied by a small structural distortion. We show that this distortion is not tetragonal as suggested previously, but is most likely rhombohedral. Below ${mathit{T}}_{mathit{N}2}$, ensuremath{chi}(T) is anisotropic; our data suggest that in this range ensuremath{chi}(T) is dominated by next-nearest-neighbor exchange interactions." @default.
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- W2092560165 date "1995-08-01" @default.
- W2092560165 modified "2023-09-26" @default.
- W2092560165 title "Surface and bulk magnetic properties of pyrite<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:mrow><mml:msub><mml:mrow><mml:mi mathvariant=normal>NiS</mml:mi></mml:mrow><mml:mrow><mml:mn>2</mml:mn></mml:mrow></mml:msub></mml:mrow></mml:math>: Magnetization and neutron-scattering studies" @default.
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- W2092560165 doi "https://doi.org/10.1103/physrevb.52.3555" @default.
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