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- W2092634189 abstract "Abstract The state-selected reaction of CH(X2Πν″ = 0, 1) with H2 has been studied, in which CH was generated by IRMPD of a precursor gas, CH3OH. The subsequent evolution of CH (ν″ = 0, 1) was monitored by the sensitive LIF technique. For the ground state and vibrationally excited state CH, the reaction with H2 is found to depend on the total pressure in the sample cell at room temperature, which suggests that the reaction proceeds through an intermediate adduct, CH3. The backward dissociation process is found to depend on the buffer pressure, which can be rationalized via a collision-induced backward dissociation. The decay rates of CH (ν″ = 0, 1) due to collisions with H2 and Ar at a buffer pressure of 10 Torr are kH2 (ν″ = 1) = (2.3±0.1) × 10−1 cm3 molecule−1 s−1 and kAr (ν″ = 1) = (4.4±0.1) × 10−13 cm3 molecule−1 s−1. Possible effects of the vibrational excitation on the reaction rate of CH (ν″ = 1) are discussed." @default.
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- W2092634189 date "1989-02-01" @default.
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- W2092634189 title "State-selected reaction and relaxation of CH with H2" @default.
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- W2092634189 doi "https://doi.org/10.1016/0301-0104(89)87059-4" @default.
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