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- W2092699323 abstract "The effect of surfactant micelles on the acid-catalyzed dissociation of NO from diazeniumdiolate ions of structure R1R2N[N(O)NO]- has been examined in phosphate-buffered solutions at 37 °C. The reaction behavior of zwitterionic substrates [2, R1 = R2 = H2N(CH2)2; 3, R1 = R2 = H2N(CH2)3; 4, R1 = n-Pr, R2 = H2N(CH2)3; 5, R1 = H2N(CH2)3, R2 = H2N(CH2)3NH(CH2)4] and anionic substrates [1, R1 = R2 = Et; 6, R1 = R2 = n-Pr] has been compared. All but DEA/NO (1) are catalyzed by anionic micelles of sodium dodecyl sulfate (SDS) but are unaffected by the presence of cationic cetyltrimethylammonium bromide or the zwitterionic surfactant 3-(N-dodecyl-N,N-dimethylammonio)-1-propanesulfonate (lauryl sulfobetaine). Catalysis by sodium decylphosphonate micelles has also been demonstrated for 2 (DETA/NO). The surfactant-mediated catalysis is discussed in terms of a distribution model with simultaneous reaction in the water and micellar pseudophases. Binding constants (Ks) for diazeniumdiolate association with the surfacta..." @default.
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- W2092699323 date "2003-01-16" @default.
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- W2092699323 title "Micellar Catalysis of Nitric Oxide Dissociation from Diazeniumdiolates" @default.
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- W2092699323 doi "https://doi.org/10.1021/la020889s" @default.
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