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• W2092866508 abstract "The electron-transfer capacity of molecular rectangle ions [Pt(II)(4)(PEt(3))(8)(mu-anth(2-))(2)(mu-L)(2)](4+) with anth = anthracene-1,8-diyl and L = 4,4'-bipyridine (bp) or 1,2-bis(4-pyridyl)ethene (bpe) was investigated in acetonitrile and dichloromethane using cyclic voltammetry, EPR, and UV-vis-near-IR spectroelectrochemistry. The compounds can be reversibly reduced, first in a two-electron process and then via two closely separated one-electron steps. Oxidation was also possible at rather low potentials in a reversible two-electron step, followed by an electrochemically irreversible process. The spectroscopic results indicate reduction at the neutral acceptor ligands L and oxidation at the formally dianionic anthracene clips. In contrast, the prototypical molecular square ([Pt(triphos)(mu-bp)](4))(8+) undergoes only irreversible reduction." @default.
• W2092866508 created "2016-06-24" @default.
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• W2092866508 date "2002-07-01" @default.
• W2092866508 modified "2023-10-16" @default.
• W2092866508 title "Metalla-Supramolecular Rectangles as Electron Reservoirs for Multielectron Reduction and Oxidation" @default.
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• W2092866508 doi "https://doi.org/10.1021/ic020122n" @default.
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