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- W2093196026 abstract "A theory of rotational relaxation of spherical top molecules in an inert gas is given, under the assumption that the molecules and atoms collide as rough spheres. Some general aspects of relaxation theory are first discussed and a theorem is presented which, under some circumstances, allows the problem to be greatly simplified. The rotational relaxation problem is then solved both for two- and three-dimensional systems. If I is the moment of inertia of the rotating molecule, m the reduced mass of the atom-molecule system, and a the sum of the atomic and molecular radii, and if b=I/ma2, then the most important result of the three-dimensional theory is that Zeff=38(1+b)2/b, where Zeff is the number of collisions suffered by each molecule in a time equal to the relaxation time. This is the analog of a result previously derived by Wang Chang and Uhlenbeck for self-relaxation in the pure molecular gas. Values of Zeff are calculated for a variety of mixtures of spherical top molecules with inert gases." @default.
- W2093196026 created "2016-06-24" @default.
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- W2093196026 date "1960-03-01" @default.
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- W2093196026 title "Rotational Relaxation of Rough Spheres" @default.
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- W2093196026 doi "https://doi.org/10.1063/1.1730817" @default.
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