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- W2093204027 abstract "We use neutron scattering to study the ${mathrm{Pr}}^{3+}$ crystalline electric field (CEF) excitations in the filled skutterudite $mathrm{Pr}{mathrm{Os}}_{4}{mathrm{As}}_{12}$. By comparing the observed levels and their strengths under neutron excitation with the theoretical spectrum and neutron excitation intensities, we identify the ${mathrm{Pr}}^{3+}$ CEF levels and show that the ground state is a magnetic ${ensuremath{Gamma}}_{4}^{(2)}$ triplet, and the excited states ${ensuremath{Gamma}}_{1}$, ${ensuremath{Gamma}}_{4}^{(1)}$, and ${ensuremath{Gamma}}_{23}$ are at 0.4, 13, and $23phantom{rule{0.3em}{0ex}}mathrm{meV}$, respectively. A comparison of the observed CEF levels in $mathrm{Pr}{mathrm{Os}}_{4}{mathrm{As}}_{12}$ with the heavy fermion superconductor $mathrm{Pr}{mathrm{Os}}_{4}{mathrm{Sb}}_{12}$ reveals the microscopic origin of the differences in the ground states of these two filled skutterudites." @default.
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- W2093204027 date "2008-03-25" @default.
- W2093204027 modified "2023-09-28" @default.
- W2093204027 title "Inelastic neutron scattering study of crystal field levels inPrOs4As12" @default.
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- W2093204027 doi "https://doi.org/10.1103/physrevb.77.094428" @default.
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