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- W2093277881 abstract "Photoionization is observed in HBr (at 300 K) below the adiabatic threshold. The photoion yield curve has structure, and is independent of both pressure and electric field over a large range. The peaks can be simulated rather well by a model which assumes rotational autoionization, with ΔN≂−4. This model does not exclude concomitant processes with ΔN=−1,−2,−3. A formal theory is also presented, which describes ΔN=−4 as occurring through successive quadrupole transitions, in second-order perturbation theory. A tentative conclusion is drawn, based on preliminary studies of other molecules, that a type of rotational autoionization can occur in heteronuclear diatomic molecules without an electric field, and in homonuclear diatomic molecules with such a field. The photoionization of DBr has been studied with similar conditions. A corresponding simulation is in good agreement with the observed structure below the adiabatic threshold. In addition, one peak in a triad observed in HBr above threshold, and predicted by an MQDT calculation to be absent in DBr, is still observed." @default.
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- W2093277881 date "1990-08-01" @default.
- W2093277881 modified "2023-09-25" @default.
- W2093277881 title "Photoionization of HBr and DBr near threshold" @default.
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- W2093277881 doi "https://doi.org/10.1063/1.459101" @default.
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