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• W2093290480 abstract "Coulomb explosion has been promoted in a range of doubly charged atomic and molecular clusters. In these new experiments, mass selected clusters of Ar2+n, (CO2)2+n, (H2O)2+n, (H2O)nH2+2, (CH3CN)nH2+2, and (C6H6)2+n have been subjected to collisional activation with a background gas. For species close to the Coulomb cutoff, each collision removes sufficient atoms or molecules (approximately six) as to render the clusters unstable. As a result, charge separation occurs and part (≂30%) of the Coulomb repulsion energy is released in the form of center of mass kinetic energy in the fragments. The remaining Coulomb energy appears as internal excitation in the fragments and subsequently leads to extensive evaporation. It is shown that the latter process is continuing even 10−6 s after Coulomb explosion. All the molecular systems studied show evidence of asymmetric charge separation, with some singly charged fragments containing up to 65% of the initial cluster mass. A detailed quantitative analysis of the results is made difficult by the very broad range of fragment ion sizes." @default.
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• W2093290480 date "1992-01-01" @default.
• W2093290480 modified "2023-09-26" @default.
• W2093290480 title "Observations of Coulomb explosion in doubly charged atomic and molecular clusters" @default.
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• W2093290480 doi "https://doi.org/10.1063/1.462851" @default.
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