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- W2093480557 abstract "A general method for producing low-fouling biomaterials on any surface by surface-initiated grafting of polymer brushes is presented. Our procedure uses radiofrequency glow discharge thin film deposition followed by macro-initiator coupling and then surface-initiated atom transfer radical polymerization (SI-ATRP) to prepare neutral polymer brushes on planar substrates. Coatings were produced on substrates with variable interfacial composition and mechanical properties such as hard inorganic/metal substrates (silicon and gold) or flexible (perfluorinated poly(ethylene-co-propylene) film) and rigid (microtitre plates) polymeric materials. First, surfaces were functionalized via deposition of an allylamine plasma polymer thin film followed by covalent coupling of a macro-initiator composed partly of ATRP initiator groups. Successful grafting of a hydrophilic polymer layer was achieved by SI-ATRP of N,N'-dimethylacrylamide in aqueous media at room temperature. We exemplified how this method could be used to create surface coatings with significantly reduced protein adsorption on different material substrates. Protein binding experiments using labelled human serum albumin on grafted materials resulted in quantitative evidence for low-fouling compared to control surfaces." @default.
- W2093480557 created "2016-06-24" @default.
- W2093480557 creator A5024023946 @default.
- W2093480557 creator A5051306293 @default.
- W2093480557 creator A5070888129 @default.
- W2093480557 date "2012-02-01" @default.
- W2093480557 modified "2023-10-05" @default.
- W2093480557 title "A substrate-independent method for surface grafting polymer layers by atom transfer radical polymerization: Reduction of protein adsorption" @default.
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- W2093480557 doi "https://doi.org/10.1016/j.actbio.2011.10.006" @default.
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