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- W2093576887 abstract "Abstract Isothermal oscillations developed during N 2 O decomposition over Co-ZSM-5 catalysts with different Si/Al ratios have been investigated. Spontaneous oscillations were observed between 350 and 450 °C. The maximum amplitude has been obtained for the catalysts having Si/Al of 40 and 50. The activation energies of the obtained oscillations were calculated in respect to cobalt concentration. The results showed that the E a values increase linearly with an increasing Si/Al ratio of the zeolite. For Co-ZSM-5 catalyst (Si/Al = 25), increasing cobalt content in the catalyst led to a decrease in the frequency as well as the amplitude of the oscillations. Meanwhile, the increase in the E a values was observed. The calculated reaction rate was found to be first order with respect to nitrous oxide concentration. Moreover, the developed oscillations were found to be sensitive to inlet N 2 O concentration, catalyst weight and milling time duration. Decreasing the N 2 O inlet concentration as well as the catalyst weight and increasing the milling time would lead to a quenching of the developed oscillations." @default.
- W2093576887 created "2016-06-24" @default.
- W2093576887 creator A5013045538 @default.
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- W2093576887 date "2009-01-01" @default.
- W2093576887 modified "2023-09-26" @default.
- W2093576887 title "Self oscillatory behaviour in N2O decomposition over Co-ZSM-5 catalysts" @default.
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- W2093576887 doi "https://doi.org/10.1016/j.apcatb.2008.07.002" @default.
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