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- W2093661431 abstract "The onset of dimerization in organic mixed-stack compounds allows the appearance of the otherwise symmetric phonons in the absorption spectra. A general theoretical framework shows that the most sensitive effect arises when symmetric and antisymmetric modes have nearby frequencies; the growth of dimerization then leads to gradual transfer of absorption intensity, from the antisymmetric mode to the symmetric one. Absorption data on tetramethyl-$p$-phenylene-diamine chloranil show this feature and thereby demonstrate the onset of dimerization below AA{}250 K. The transition involves a small and continuous change in ionicity." @default.
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- W2093661431 date "1986-10-15" @default.
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- W2093661431 title "Spectroscopy of dimerization in organic mixed-stack compounds and tetramethyl-<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:mi>p</mml:mi></mml:math>-phenylene-diamine chloranil" @default.
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- W2093661431 doi "https://doi.org/10.1103/physrevb.34.6056" @default.
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