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• W2093674811 abstract "Peroxynitrite (ONOO-) reacts rapidly with excess of CO2 to yield in water 30−35% CO3•- and •NO2 radicals, which oxidize 2,2‘-azino-bis(3-ethylbenzthiazoline-6-sulfonic acid) (ABTS) and ferrocyanide. The yield of ABTS+ decreased upon increasing the glycerol concentration, independent of [ABTS]o, and was, within experimental error, identical to that of ferricyanide at the same concentration of glycerol. These results demonstrate that the decrease in the oxidation yields upon increasing the glycerol concentration does not result from a competition between glycerol and ABTS/ferrocyanide for the oxidizing radicals but is due to an increase in viscosity. The oxidation yields were less affected by poly(ethylene glycol) than by glycerol, though the macroscopic viscosities of the polymer solutions were much higher. We conclude that the mechanism of the decomposition of peroxynitrite in the presence of CO2 takes place through the formation of CO3•- and •NO2 in a solvent cage. In addition, in the glycerol−water syst..." @default.
• W2093674811 created "2016-06-24" @default.
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• W2093674811 date "1999-03-01" @default.
• W2093674811 modified "2023-09-26" @default.
• W2093674811 title "Viscosity Effects on the Reaction of Peroxynitrite with CO₂: Evidence for Radical Formation in a Solvent Cage" @default.
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• W2093674811 doi "https://doi.org/10.1021/ja9822254" @default.
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