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- W2093858031 abstract "The energy content and correlation of vectorial properties of the OH fragment photoejected by methyl hydroperoxide (CH3OOH) at 266 nm are probed by laser excitation, polarization, and high-resolution sub-Doppler spectroscopy. The nascent OH is found to be vibrationally cold and the rotational distribution peaks at ∼N=6. Polarization dependence of the fragment Doppler profiles and nonequilibrium Λ-doublet populations show that, at high rotational energy, the velocity vector of the OH fragment has a preference to be perpendicular to the planes of rotation of the nuclei and the half-filled 2pπ orbital. The fragment angular distribution indicates that dissociation of the parent excited state is fairly prompt, with a lifetime of ∼250 fs." @default.
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- W2093858031 date "1990-12-15" @default.
- W2093858031 modified "2023-09-24" @default.
- W2093858031 title "Photodissociation of methyl hydroperoxide at 266 nm: Vector correlations and energy distribution in the OH fragment" @default.
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- W2093858031 doi "https://doi.org/10.1063/1.459260" @default.
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