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• W2093897689 abstract "We investigate the influence of a laser field, which is near-resonant to the atomic sodium 3$^2$P$_{1/2}$ $to$ 3$^2$D$_{3/2}$ transition, on the last bound levels of the A$^1Sigma^+_u$ state in Na$_2$. In a molecular beam experiment level shifts up to $approx$ 100 MHz and light induced line broadenings were observed using an optical double resonance excitation scheme. Moreover, the coupling laser can reduce the number of bound levels of the A state by one or more units, which effectively means that in the picture of a collision of a 3$^2$S$_{1/2}$ and a 3$^2$P$_{1/2}$-atom the scattering phase is altered by more than $pi$. The observed effects are interpreted as light induced couplings of the A$^1Sigma^+_u$ state, which correlates to the 3s$_{1/2}$+3p$_{1/2}$ asymptote, to the $4^1Sigma^+_g$ and $2^1Pi_g$ states at the 3s$_{1/2}$+3d$_{3/2}$ asymptote. We performed multi-channel calculations, applying the mapped Fourier grid method, which reproduce our experimentally observed level shifts well." @default.
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• W2093897689 date "2003-10-01" @default.
• W2093897689 modified "2023-10-18" @default.
• W2093897689 title "Optical manipulation of long-range interactions at the 3s + 3p asymptote of $mathsf{Na_2}$" @default.
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• W2093897689 doi "https://doi.org/10.1140/epjd/e2003-00294-2" @default.
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