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- W2093965912 abstract "We prepared two new linkers, S-functionalized adamantane derivatives 2 and 3, which bind as monolayers on polycrystalline gold. From these surface anchors, both L- and D-isomers of alanine can be grown as thin films of α-helical polypeptides directed from the gold surface by using the appropriate N-carboxyalanine anhydride. FT-IR Studies show that these layers are roughly 1000-Å thick and that, under the same growth conditions, the L-polypeptide layers grow at a rate ca. 30% greater than that of the non-natural D-amino acid. X-Ray photoelectron spectroscopy studies show that, upon equilibration, all three S-atoms of the sulfide moieties of 2 are bound to the gold surface, and that, on average, three of the four thiols of 3 are chemoadsorbed. The essential role of H2O on the surface of these films as a necessary component in these gas-phase polymerization reactions is demonstrated." @default.
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- W2093965912 date "2002-03-01" @default.
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- W2093965912 title "α-Helical Polypeptide Films Grown From Sulfide or Thiol Linkers on Gold Surfaces" @default.
- W2093965912 doi "https://doi.org/10.1002/1522-2675(200203)85:3<788::aid-hlca788>3.0.co;2-r" @default.
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