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• W2094064564 abstract "Production of synthesis gas suitable for the production of liquid fuels, chemicals, and methane by the Fischer−Tropsch (FT) synthesis process from catalytic gasification of coal has been investigated. Coal and HyperCoal were gasified in a steam and CO2 mixed environment as a gasifying agent at 700, 650, and 600 °C with K2CO3 as a catalyst. The H2/CO ratio of the synthesis gas was controlled by changing the steam/CO2 ratio of the gasifying agent. Gasification rates decreased with a decreasing temperature and an increasing CO2 fraction in the gas mixture but were high enough for practical application. The H2/CO ratio was primarily affected by the CO2 fraction in the mixed gas. Gasification rates in H2O + CO2 mixed gas were not the sum of individual C−H2O and C−CO2 pure-gas rates. The role of the water−gas shift reaction in controlling gas composition in H2O + CO2 mixed gas was investigated. The results showed that synthesis gas suitable as feedstock for dimethyl ether (DME), methanol, methane, and other chemicals production by the FT synthesis process can be produced in a single step at 700−600 °C by catalytic gasification of coal in steam/CO2 mixed gas as a gasifying agent. A single-step process to produce and control composition of synthesis gas from coal was proposed." @default.
• W2094064564 created "2016-06-24" @default.
• W2094064564 creator A5053849530 @default.
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• W2094064564 date "2009-12-23" @default.
• W2094064564 modified "2023-09-25" @default.
• W2094064564 title "Controlling the H₂/CO Ratio of the Synthesis Gas in a Single Step by Catalytically Gasifying Coal in a Steam and Carbon Dioxide Mixed Environment at Low Temperatures" @default.
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• W2094064564 doi "https://doi.org/10.1021/ef901178d" @default.
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