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• W2094177521 abstract "We demonstrate a technique that uses high-order harmonic generation in molecules to probe nuclear dynamics and structural rearrangement on a subfemtosecond time scale. The chirped nature of the electron wavepacket produced by laser ionization in a strong field gives rise to a similar chirp in the photons emitted upon electron-ion recombination. Use of this chirp in the emitted light allows information about nuclear dynamics to be gained with 100-attosecond temporal resolution, from excitation by an 8-femtosecond pulse, in a single laser shot. Measurements on molecular hydrogen and deuterium agreed well with calculations of ultrafast nuclear dynamics in the H 2 + molecule, confirming the validity of the method. We then measured harmonic spectra from CH 4 and CD 4 to demonstrate a few-femtosecond time scale for the onset of proton rearrangement in methane upon ionization." @default.
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• W2094177521 date "2006-04-21" @default.
• W2094177521 modified "2023-10-18" @default.
• W2094177521 title "Probing Proton Dynamics in Molecules on an Attosecond Time Scale" @default.
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• W2094177521 doi "https://doi.org/10.1126/science.1123904" @default.
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