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- W2094371432 abstract "The influence of the electronic asymmetry in the 1Δ(A′) and 1Δ(A″) Λ doublets of NR (R=H,D) on the photodissociation dynamics of hydrazoic acid (RN3) has been investigated. Hydrazoic acid was prepared in its first excited electronic state, Ã1A″. A variety of scalar (internal state and translational energy distribution) and vectorial (angular distribution, rotational alignment, correlation between translational and rotational motion) properties of the ejected NH or ND fragment were analyzed by Λ-doublet-specific Doppler profile measurements. While the population of the 1Δ(A′) and 1Δ(A″) states are equal, the vector correlations for both Λ sublevels are different. NR(A″) products are preferentially ejected in the original plane formed by the parent, and the recoil of NR fragments in the symmetric Δ(A′) state is preferentially perpendicular to that plane. The vector correlation between the translational and the rotational motion of the fragment also indicates a strong nonplanar dissociation geometry for NR products in the Δ(A′) state. About 50% of the ND(A′) product rotation is generated by a torsional motion, while 80% of the ND(A″) fragments are formed with J being aligned perpendicular to the recoil direction (MJ=0)." @default.
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- W2094371432 date "1992-01-01" @default.
- W2094371432 modified "2023-09-23" @default.
- W2094371432 title "Influence of the electronic asymmetry in NH (1Δ) state Λ doublets on the photodissociation dynamics of HN3 and DN3" @default.
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- W2094371432 doi "https://doi.org/10.1063/1.462477" @default.
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