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• W2094642795 endingPage "2024" @default.
• W2094642795 startingPage "2019" @default.
• W2094642795 abstract "Abstract Charge transport (CT) in a Nafion membrane containing μ-oxobis[aquabis(2,2′-bipyridine)ruthenium(III)] complex, [(bpy)2(H2O)RuORu(H2O)(bpy)2]4+ (bpy=2,2′-bipyridine, abbreviated to RuIIIORuIII) was investigated by potential-step chronocoulospectrometry (PSCCS). Electrochemical reduction of RuIIIORuIII in the membrane occurred irreversibly to form [Ru(bpy)2(OH2)2]2+ monomer. The CT by reduction of RuIIIORuIII in the membrane was suggested to take place by physical displacement of the complex, which is quite different from the mechanism in the CT by oxidation of RuIIIORuIII in the same membrane in which charge is transported by charge hopping based on reversible redox reaction between RuIIIORuIII and RuIIIORuIV. The fractions of the electrochemically reacted complex in the membrane for the oxidative CT was dependent on the complex concentration, and the yield was low (maximum fraction=0.42 at 0.87 M) relative to the reductive CT. By contrast, the fraction for the reductive CT was independent of the concentration over 0.12 M and close to unity. The different concentration dependence of the fraction was discussed related to the difference in the CT mechanism." @default.
• W2094642795 created "2016-06-24" @default.
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• W2094642795 date "2002-05-01" @default.
• W2094642795 modified "2023-09-23" @default.
• W2094642795 title "Mechanistic comparison between oxidative and reductive charge transport by [(bpy)2(H2O)RuORu(H2O)(bpy)2]4+ confined in a Nafion membrane as studied by potential-step chronocoulospectrometry" @default.
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• W2094642795 doi "https://doi.org/10.1016/s0013-4686(02)00105-6" @default.
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