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- W2094805502 abstract "We describe a method to probe the spectral fluctuations of a transition over broad ranges of frequencies and timescales with the high spectral resolution of Fourier spectroscopy, and a temporal resolution as high as the excited state lifetime, even in the limit of very low photocounting rates. The method derives from a simple relation between the fluorescence spectral dynamics of a single radi-ating dipole and its fluorescence intensity correlations at the outputs of a continuously scanning Michelson interferometer. These findings define an approach to investigate the fast fluorescence spectral dynamics of single molecules and other faint light sources beyond the time-resolution capabilities of standard spectroscopy experiments." @default.
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- W2094805502 date "2006-01-01" @default.
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- W2094805502 title "Photon-correlation Fourier spectroscopy" @default.
- W2094805502 doi "https://doi.org/10.1364/oe.14.006333" @default.
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