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• W2094912059 abstract "The stability of highly charged gas phase metal ion solvates [M(Sol)n]z+ (z>2) is discussed based on a simple electrostatic model and density functional theory computations. It is often assumed that the observation of such ions will be increasingly difficult as z increases because they will be less and less stable, i.e., that they will have an increasing tendency to undergo spontaneous charge-separating dissociation into fragment ions of lower charge. It is shown here that for carefully chosen metal ions such as Zr4+, this need not be the case—many highly charged metal solvates, such as [Zr(CH3CN)]4+, should exist with very significant metastable lifetimes. However, it may be difficult to isolate and identify such ions experimentally without the interference of competing processes such as charge-separating dissociation or charge reduction through electron transfer during collisions with other molecules in the ion source." @default.
• W2094912059 created "2016-06-24" @default.
• W2094912059 creator A5010164558 @default.
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• W2094912059 date "2003-08-01" @default.
• W2094912059 modified "2023-10-11" @default.
• W2094912059 title "Microsolvation of metal ions: on the stability of [Zr(CH3CN)]4+ and other multiply charged ions" @default.
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• W2094912059 doi "https://doi.org/10.1016/s1387-3806(03)00160-x" @default.
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