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- W2095388884 abstract "Abstract A novel crystalline bis( n -undecylammonium) tetrachlorozincate (C 11 H 23 NH 3 ) 2 ZnCl 4 (s) was synthesized by liquid phase reaction. X-ray single crystal diffraction technique, chemical analysis, and elementary analysis were used to determine crystal structure and chemical composition of the complex. Lattice potential energy was calculated to be U POT = 873.05 kJ · mol −1 from crystallographic data. Molar enthalpies of dissolution of the compound at different molalities in the double-distilled water were measured with an isoperibol solution-reaction calorimeter at T = 298.15 K. On the basis of Pitzer’s electrolyte solution theory, molar enthalpy of dissolution of (C 11 H 23 NH 3 ) 2 ZnCl 4 (s) at infinite dilution was calculated to be Δ s H m ∞ = (42.67 ± 0.340) kJ · mol −1 , and sums of Pitzer parameters 4 β C 11 H 23 NH 3 ,Cl ( 0 ) L + 2 β Zn,Cl ( 0 ) L + θ C 11 H 23 NH 3 ,Zn L and 2 β C 11 H 23 NH 3 ,Cl ( 1 ) L + β Zn,Cl ( 1 ) L were obtained. In addition, the molar enthalpy of hydration of the cation [C 11 H 23 NH 3 ] + in the complex (C 11 H 23 NH 3 ) 2 ZnCl 4 (s) was calculated to be Δ H + = −(25.52 ± 0.878) kJ · mol −1 by designing a thermochemical cycle based on lattice potential energy and molar enthalpy of dissolution of the title complex at infinite dilution." @default.
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- W2095388884 date "2012-11-01" @default.
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- W2095388884 title "Crystal structure and thermochemical properties of bis(n-undecylammonium) tetrachlorozincate (C11H23NH3)2ZnCl4(s)" @default.
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- W2095388884 doi "https://doi.org/10.1016/j.jct.2012.03.035" @default.
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