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• W2095397230 endingPage "5361" @default.
• W2095397230 startingPage "5353" @default.
• W2095397230 abstract "Interferences in vibrational wave packets of Br2 molecules are controlled in the presence of a solid Ar environment that provides decoherence. By applying a negatively or positively chirped excitation pulse, one can set the clock backward, respectively forward, in the wave packet propagation. Based on this mechanism, we present a general scheme to record vibrational decoherence. Wave packets are spatially focused at Topt by applying negatively chirped pulses. From the focussing contrast, we determine a vibrational dephasing time on the B state of Tvibdeph = 3 ps. We use positively chirped pulses to bring the formation of fractional revival structures forward with respect to Tvibdeph. By exciting four vibrational levels with such a pulse, we observe a 1/6 revival indicating the vibrational coherence time T4deph for exactly four levels. The required chirp prolongs the pulse duration by a factor of ten to Δτ = 300 fs. Electronic dephasing Teldeph restricts the revival control efficiency to parts of the pulse with Δτ < Teldeph, which allows to derive Teldeph > 300 fs." @default.
• W2095397230 created "2016-06-24" @default.
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• W2095397230 date "2004-01-01" @default.
• W2095397230 modified "2023-10-16" @default.
• W2095397230 title "Controlling vibrational wave packet revivals in condensed phase: Dispersion and coherence for Br₂in solid Ar" @default.
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• W2095397230 doi "https://doi.org/10.1039/b413635g" @default.
• W2095397230 hasPublicationYear "2004" @default.
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