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• W2095415672 abstract "The framework presented here was developed to provide an objective mechanism for incorporating the primary structural aspects of a polymer in predicting physical properties, especially mechanical and optical properties, of networks. It incorporates the effective chain distributions, obtained by Nanavati et al. from vector-length and polarizability distributions of statistical segments. The efficacy of this approach has been tested by comparing the predictions to published experimental data for networks of poly(cis-isoprene) and polyethylene, with primarily a single fitted parameter, namely, the effective chemical crosslink density. The improvement which can be obtained through an additional empirical parameter to incorporate the effects of entanglement-like topological constraints has also been explored. The best predictions are obtained through a combination of the current formulation and Treloar’s postulate of a constant chain vector length in the undeformed state. With just one (or two) fitted parameters, excellent predictions have been obtained of stress–deformation over a broad range of deformation. Also, the polarizability–deformation relationships, obtained without any additional fitted parameter, have been found to be very good. The results show that, by coupling molecular modeling with classical analysis of network characteristics, constitutive relations for rheological, optical and dielectric properties of polymer networks can be obtained, with due consideration of their primary structures." @default.
• W2095415672 created "2016-06-24" @default.
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• W2095415672 date "1999-06-01" @default.
• W2095415672 modified "2023-09-26" @default.
• W2095415672 title "Elastic and photoelastic relationships for crosslinked polymer networks: a statistical segment approach" @default.
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• W2095415672 doi "https://doi.org/10.1016/s1089-3156(99)00011-2" @default.
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