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• W2095427424 startingPage "2360" @default.
• W2095427424 abstract "There is an increased need for alginate materials with both enhanced and controllable mechanical properties in the fields of food, pharmaceutical and specialty applications. In the present work, well-characterized algal polymers and mannuronan were enzymatically modified using C-5 epimerases converting mannuronic acid residues to guluronic acid in the polymer chain. Composition and sequential structure of controls and epimerized alginates were analyzed by 1H NMR spectroscopy. Mechanical properties of Ca-alginate gels were further examined giving Young’s modulus, syneresis, rupture strength, and elasticity of the gels. Both mechanical strength and elasticity of hydrogels could be improved and manipulated by epimerization. In particular, alternating sequences were found to play an important role for the final mechanical properties of alginate gels, and interestingly, a pure polyalternating sample resulted in gels with extremely high syneresis and rupture strength. In conclusion, enzymatic modification was shown to be a valuable tool in modifying the mechanical properties of alginates in a highly specific manner." @default.
• W2095427424 created "2016-06-24" @default.
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• W2095427424 date "2008-08-15" @default.
• W2095427424 modified "2023-10-14" @default.
• W2095427424 title "Mechanical Properties of C-5 Epimerized Alginates" @default.
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• W2095427424 doi "https://doi.org/10.1021/bm8003572" @default.
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