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- W2095480706 abstract "A detailed investigation of chemi-ionization and chemi-luminescence in H 2 /O 2 /N 2 +C 2 N 2 flames has led to the following conclusions: o (a) A single molecule of C 2 N 2 is required for the formation of an ion or excited species such as CN * or NH * . (b) The very high ionic yield and the large over-all activation energy suggest a bimolecular process for the primary ionization. The variation of the ionic yield with pressure shows that the overall order of the chemi-ionization process is greater by one than that of the combustion process. (c) Since the thickness of the flame front depends on the pressure as P −0.7 , the over-all combustion reaction corresponds to a 1.4 order, and therefore a 2.4 apparent order for the over-all chemi-ionization reaction can be deduced. (d) These results lead us to propose the following mechanism for the formation reactions of the primary ion (NO + ): CN+O→N( 2 P )+CO CN+O→N( 2 D )+CO N( 2 P )→N( 2 D )+ hν N( 2 P )+O→NO + + e − N( 2 D )+O→NO + + e − Such a mechanism accounts for all our experimental results for NO + and the other ionic species detected by mass spectrometry. Some data for the excited CN-radical are also discussed." @default.
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- W2095480706 date "1975-01-01" @default.
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- W2095480706 title "Mechanism of ion and emitter formation due to cyanogen in hydrogen-oxygen-nitrogen flames" @default.
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