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• W2098989524 abstract "A polymeric gel can imbibe solvent and swell. Besides the dilatational mode of deformation, which involves long-range solvent migration, a gel may also undergo volume-conserved deformation. For a macroscopic gel with covalent cross-links, the volume-conserved deformation is usually much faster. However, these two modes are coupled for deformation at the microscopic level and for gels containing physical cross-links or large solvent molecules. In this paper, we seek to formulate a unified theoretical framework for the transient behaviour of polymeric gels to account for both solvent migration and viscoelastic deformation. Under this framework, we further develop a simple material model, and implement it into a finite-element code for numerical calculations. By simultaneously tracking the solvent migration and motion of polymer network, we evolve the inhomogeneous fields of stress and chemical potential. Several initial-boundary-value problems are solved as illustrative examples. For macroscopic gels with low viscosity, the time scales for viscoelasticity and poroelasticity are separated, and the long-term behaviour is just as that predicted by a poroelastic model. For structures or processes involving sizes comparable to the intrinsic length of a material, the viscoelasticity and poroelasticity must be considered simultaneously, especially when studying impact responses." @default.
• W2098989524 created "2016-06-24" @default.
• W2098989524 creator A5019263952 @default.
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• W2098989524 date "2012-08-29" @default.
• W2098989524 modified "2023-10-14" @default.
• W2098989524 title "A visco-poroelastic theory for polymeric gels" @default.
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• W2098989524 doi "https://doi.org/10.1098/rspa.2012.0385" @default.
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