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- W2099377557 abstract "• Positive and negative TOF-SIMS spectra by 10–20 keV Ga + bombardment of [C n mim][Tf 2 N], where n = 2, 4, 6, 8, were measured. • The predominant peaks were intact cation [C n mim] + and anion fragment F − . • The sum intensity of positive cation fragments increased with an increase in the alkyl chain length ( n -value). • Ion-induced fragmentation of anion decreased with an increase of the n -value and with a decrease in the projectile energy. An upgraded TOF-SIMS VG Ionex IX23LS was used to study the fragmentation patterns of a series of asymmetric imidazolium ionic liquids [C n mim][Tf 2 N], where n = 2, 4, 6, and 8, under bombardment by Ga + ions with energies of 10–20 keV. Analysis of positive and negative secondary ion mass spectra showed that fragmentation of cations and anion proceeds via both one- and two-bond cleavage of molecular backbone. In addition, formation of methylene adducts [C n mim(CH 2 ) x ] + , where x = 1–3, and associates containing anion constituents [C n mimO] + and [C n mimF] + was revealed. Lengthening of alkyl chain was found to result in a stronger fragmentation of cations, while the extent of ion-induced fragmentation of anion decreased with an increase of the n -value and with a decrease in the projectile impact energy." @default.
- W2099377557 created "2016-06-24" @default.
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- W2099377557 date "2013-11-01" @default.
- W2099377557 modified "2023-09-24" @default.
- W2099377557 title "Ion-induced fragmentation of imidazolium ionic liquids: TOF-SIMS study" @default.
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- W2099377557 doi "https://doi.org/10.1016/j.ijms.2013.05.029" @default.
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