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• W2099558301 abstract "This work addresses the remediation of nitrate-contaminated water using electrodes made of Ebonex (a titanium oxide ceramic with a wide range of potential stability). The objective was the complete denitrification of solutions containing nitrate ion. Denitrification was achieved in about 50% yield with unreactive supporting electrolytes when Ebonex was used as both cathode and anode, the remaining product being ammonia. Ammonia could be re-oxidized at the Ebonex anode, but this was much less efficient than the reduction step. A more efficient electrolytic denitrification was possible for solutions containing chloride; this is oxidized anodically to hypochlorite, which then oxidizes ammonia chemically to N 2 . The overall rate of denitrification was highest at moderate concentrations of chloride ion, because hypochlorite also re-oxidizes reduction intermediates such as nitrite back to nitrate. Complete denitrification was achieved at all stages of the reaction using Ebonex cathode and a dimensionally stable anode based on Ti/IrO 2 or Ti/RuO 2 , because the DSA oxidizes chloride ion more efficiently than Ebonex. Cathode fouling by water sources that are high in hardness cations can be prevented by using one DSA and a pair of Ebonex electrodes that undergo periodic polarity reversal." @default.
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• W2099558301 date "2012-08-01" @default.
• W2099558301 modified "2023-10-14" @default.
• W2099558301 title "The use of Ebonex electrodes for the electrochemical removal of nitrate ion from water" @default.
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• W2099558301 doi "https://doi.org/10.1139/v2012-048" @default.
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