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• W2100099528 abstract "Results from a recent quantum Monte Carlo (QMC) study [P. B. Chakraborty et al., Phys. Rev. B 70, 144411 (2004)] of a model of the ${text{LiHoF}}_{4}$ Ising magnetic material in an external transverse magnetic field, ${B}_{x}$, show a discrepancy with experimental results, even for small ${B}_{x}$ where quantum fluctuations are small. This discrepancy persists asymptotically close to the classical ferromagnet to paramagnet phase transition. In this paper, we numerically reinvestigate the temperature $T$ versus transverse-field phase diagram of ${text{LiHoF}}_{4}$ in the regime of weak ${B}_{x}$. In this regime, starting from an effective low-energy spin-1/2 description of ${text{LiHoF}}_{4}$, we apply a cumulant expansion to derive an effective temperature-dependent classical Hamiltonian that incorporates perturbatively the small quantum fluctuations in the vicinity of the classical phase transition at ${B}_{x}=0$. Via this effective classical Hamiltonian, we study the ${B}_{x}text{ensuremath{-}}T$ phase diagram via classical Monte Carlo simulations. In particular, we investigate the influence on the phase diagram of various effects that may be at the source of the discrepancy between the previous QMC results and the experimental ones. In particular, we consider two different ways of handling the long-range dipole-dipole interactions and explore how the ${B}_{x}text{ensuremath{-}}T$ phase diagram is modified when using different microscopic crystal-field Hamiltonians. The main conclusion of our work is that we fully reproduce the previous QMC results at small ${B}_{x}$. Unfortunately, none of the modifications to the microscopic Hamiltonian that we explore are able to provide a ${B}_{x}text{ensuremath{-}}T$ phase diagram compatible with the experiments in the quasiclassical small ${B}_{x}$ regime." @default.
• W2100099528 created "2016-06-24" @default.
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• W2100099528 date "2008-11-11" @default.
• W2100099528 modified "2023-09-23" @default.
• W2100099528 title "Perturbative quantum Monte Carlo study of<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:mrow><mml:msub><mml:mrow><mml:mtext>LiHoF</mml:mtext></mml:mrow><mml:mn>4</mml:mn></mml:msub></mml:mrow></mml:math>in a transverse magnetic field" @default.
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• W2100099528 doi "https://doi.org/10.1103/physrevb.78.184408" @default.
• W2100099528 hasPublicationYear "2008" @default.
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