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• W2100226936 abstract "A series of Pr(1-x)Ca(x)CoO(3) samples were prepared using a novel molten salt reaction that is convenient to obtain single phases avoiding aggregates compared to conventional solid state reactions. The formation reaction was monitored by X-ray diffraction combined with thermal analysis, and all samples were characterized by X-ray diffraction, scanning electron microscopy, Fourier transform infrared spectroscopy, and alternating current impedance. It is demonstrated that all Pr(1-x)Ca(x)CoO(3) samples crystallized in a pure orthorhombic perovskite structure. By increasing the doping level, the symmetry of the orthorhombic structure was enhanced, and is followed by an increase in the population of Co(3+) in the intermediate spin state. All samples exhibited typical semiconducting behavior, showing conductivities highly dependent on the Ca(2+) doping. The conduction for x = 0 shows a simple thermal activated process, which changed into a Mott's variable range hopping mechanism for x > 0. By increasing the Ca(2+) doping level, the relevant activation energy is decreased, while the density of the localized electronic state is increased." @default.
• W2100226936 created "2016-06-24" @default.
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• W2100226936 date "2011-01-01" @default.
• W2100226936 modified "2023-10-11" @default.
• W2100226936 title "Lightly doping Ca2+ in perovskite PrCoO3 for tailored spin states and electrical properties" @default.
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• W2100226936 doi "https://doi.org/10.1039/c1cp21562k" @default.
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