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- W2100692011 abstract "A number of fulvene compounds, which can polarize to give rise to intramolecular charge transfer (ICT), have been synthesized, and the second-order molecular hyperpolarizability (β)and dipole moment (µg) have been calculated by using the MOPAC program. The macroscopic non-linearity (second-harmonic generation; SHG) evaluated by the Kurtz powder method is discussed in relation to microscopic β and µg. The large β and the small µg are characteristic of these compounds and contribute to the SHG activity Among these compounds, ω-(p-methoxyphenyl)benzofulvene (MPBF) was found to exhibit large SHG activity and could be grown into large crystals. X-Ray diffraction analysis of MPBF shows non-centrosymmetrically cylindrical packing along the b-axis. The effective non-linear optical coefficient deff of MPBF, which was evaluated from the bulk crystal cut to the phase-matching direction, corresponds to the value (7.0 pm V–1) of potassium titanylphosphate (KTP), although the hardness is low (24 Vickers hardness)." @default.
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- W2100692011 date "1992-01-01" @default.
- W2100692011 modified "2023-10-16" @default.
- W2100692011 title "Micro- and macro-scopic second-order non-linear optical properties of fulvene compounds" @default.
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- W2100692011 doi "https://doi.org/10.1039/jm9920201097" @default.
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