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- W2101379022 abstract "Dielectric measurements of an epoxy resin, N, N-diglycidyl-4-glycidyloxyaniline, have been carried out in the supercooled and glassy phase over a broad frequency range (102-6 ×109 Hz). The measurements reveal electrical transport due to ionic impurities as well as three different dipolar relaxations - in addition to the - and -relaxation, a slower ´-relaxation is recognized, whose loss peak is disclosed after subtraction of the dc conductivity contribution. The glass transition is found to affect markedly the secondary relaxation, whose strength and shape parameters change across Tg. The major inference from the results concerns the existence of a transition in the dynamics, occurring some tens of degrees above Tg, in the vicinity of the temperature TS where the peaks of the - and -relaxations merge. Evidence in favour of such a transition is given by: (i) the change in the temperature dependence of the -relaxation time; (ii) independently, the change in the temperature dependence of the dc conductivity; (iii) the breakdown of the Debye-Stokes-Einstein model, replaced at lower temperatures by a fractional regime." @default.
- W2101379022 created "2016-06-24" @default.
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- W2101379022 date "1999-12-09" @default.
- W2101379022 modified "2023-10-16" @default.
- W2101379022 title "Dynamics of a glass-forming triepoxide studied by dielectric spectroscopy" @default.
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- W2101379022 doi "https://doi.org/10.1088/0953-8984/11/50/322" @default.
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