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- W2101883976 abstract "Dioxygen is used as the oxygenation agent in the rhodium-mediated conversion of nitriles into amides. The characterization of intermediate species and model compounds as well as isotope-labeling studies provided an insight into the reaction mechanism. The conversions of rhodium hydroperoxido or methylperoxido complexes with nitriles into metallacyclic rhodium-κ(2)-(N,O)-peroxyimidate compounds represent essential key steps. The former are accessible from a rhodium(III) peroxido complex and the latter represent rhodium derivatives of Payne's reagent (peroxyimidic acids)." @default.
- W2101883976 created "2016-06-24" @default.
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- W2101883976 date "2015-07-17" @default.
- W2101883976 modified "2023-10-10" @default.
- W2101883976 title "Rhodium-Mediated Oxygenation of Nitriles with Dioxygen: Isolation of Rhodium Derivatives of Peroxyimidic Acids" @default.
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- W2101883976 doi "https://doi.org/10.1002/chem.201502481" @default.
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