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- W210204857 abstract "Light induced charge separation, a decisive ingredient of photosynthesis has also been studied extensively in molecules comprising covalently bonded donor and acceptor moieties /1–4/. Unlike intermolecular charge transfer between isolated molecules in solution, which are free to diffuse, this intramolecular charge transfer takes place with a rather fixed distance and fixed relative orientation of the donor with regard to the acceptor. This makes the bonded molecules particularly suitable for mimicing the primary step in photosynthesis as well as for investigating the couplings responsible for the electron transfer. Within the Born—Oppenheimer approximation the nonadiabatic rate for charge transfer is proportional to the square of an electronic coupling term, which induces the transition from the excited electronic state to the charge transfer state, and a factor describing the nuclear rearrangements." @default.
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- W210204857 date "1990-01-01" @default.
- W210204857 modified "2023-09-27" @default.
- W210204857 title "Electronic Couplings for Light Induced Charge Transfer in Covalently Bonded Donor-Acceptor Systems" @default.
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- W210204857 doi "https://doi.org/10.1007/978-3-642-61297-8_35" @default.
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