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- W2102732010 abstract "The relationship between electronic and atomic structure of quantum confined objects is a key issue in nanoscience. We performed low-energy electron diffraction to determine the surface relaxations of ultrathin Pb films on $mathrm{Si}(111)7ifmmodetimeselsetexttimesfi{}7$ with thicknesses ranging from four to nine atomic layers. The results indicate a contraction of the first interlayer spacing ${d}_{12}$ for all films. The ${d}_{12}$ contraction exhibits a small bilayer modulation as a function of thickness, indicative of a quantum size effect. The oscillatory relaxations furthermore suggest an interesting correlation with the work function oscillations predicted from density functional theory [Wei and Chou, Phys. Rev. B 66, 233408 (2002)] and can be understood qualitatively on the basis of the jellium model." @default.
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- W2102732010 date "2005-10-31" @default.
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- W2102732010 title "Surface relaxations in quantum-confined Pb" @default.
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- W2102732010 doi "https://doi.org/10.1103/physrevb.72.155442" @default.
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