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- W2102952365 abstract "A supramolecular complex [Ru(dcb)2(α-CD-5-bpy)]Cl2 (1-α-CD) (dcb = 4,4′-dicarboxyl-2,2′-bipyridine, α-CD-5-bpy = 6-mono[5-methyl(5′-methyl-2,2′-bipyridyl)]-permethylated α-CD) (CD: cyclodextrin) based on a ruthenium tris-bipyridyl core with an appended α-CD cavity is designed and synthesised, in order to facilitate dye/redox couple interaction and dye regeneration in nanocrystalline TiO2 solar cells. The luminescent complex is fully characterized and anchored on mesoporous titania electrodes showing increased power-conversion efficiency in solid-state dye-sensitized solar cells using a composite polymer electrolyte. Direct comparison of the properties of the CD complex with an analogous ruthenium complex [Ru(dcb)2(5,5′-dmbpy)]Cl2 (2) (5,5′-dmbpy = 5,5′-dimethylbipyridine) without the CD cavity reveals that the photovoltaic performance of 1-α-CD is enhanced by about 40 % compared to 2. Independent studies have shown complexation of the iodide redox couple to the CD in 1-α-CD. These results indicate that the CD moiety is able to act as a mediator and fine tune the photoelectrode/electrolyte interface." @default.
- W2102952365 created "2016-06-24" @default.
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- W2102952365 date "2007-01-05" @default.
- W2102952365 modified "2023-10-06" @default.
- W2102952365 title "Functional Supramolecular Ruthenium Cyclodextrin Dyes for Nanocrystalline Solar Cells" @default.
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- W2102952365 doi "https://doi.org/10.1002/adfm.200600188" @default.
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