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- W2103010783 abstract "So far unobserved in the 12C17O isotopologue, the 1−υ″ progression of the Ångström (B1Σ+–A1Π) band system was recorded under high resolution in the 17,200–22,950 cm−1 spectral region as an emission spectrum using high-accuracy dispersive optical spectroscopy. The 12C17O molecules were formed and excited in two steps in a stainless steel hollow-cathode lamp with two anodes. The emission from the discharge was observed with a plane-grating spectrograph and recorded by a photomultiplier tube. In the studied region, the full rotational structure of the 1–1 and 1–5 bands of the B–A system was observed, in total 114 spectral emission lines up to J″=21. All those lines were precisely measured with an estimated accuracy of about 0.0030 cm−1, and rotationally analyzed. As a result, many molecular constants were determined for the B1Σ+ and A1Π states in the 12C17O isotopologue. In this paper we have also presented the results of calculations concerning RKR turning points, Franck–Condon factors, relative intensities, and r-centroids for the Ångström band system in the 12C17O molecule. We have also determined the value of the ΔG1/2 vibrational quantum, the isotope shifts, as well as the main, isotopically invariant parameters of the B1Σ+ Rydberg state in the CO molecule within the Born–Oppenheimer approximation. For the A1Π, υ=5 state, considerable irregularities of the rotational structure have been observed and analyzed in detail. Suspected candidates responsible for these perturbations have been identified. The B1Σ+, υ=1 state has been thoroughly analyzed in terms of possible perturbations and it emerged to be completely regular in the 12C17O molecule up to the observed maximum J value." @default.
- W2103010783 created "2016-06-24" @default.
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- W2103010783 date "2014-06-01" @default.
- W2103010783 modified "2023-09-28" @default.
- W2103010783 title "First analysis of the B1Σ+ (υ=1) Rydberg state in the lesser-abundant 12C17O isotopologue on the basis of the 1–υ″ progression of the Ångström band system" @default.
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- W2103010783 doi "https://doi.org/10.1016/j.jqsrt.2014.02.004" @default.
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